Structural, Optical, and Transport Properties of α- and β‐Ag3VO4

نویسندگان

  • V. Cloet
  • A. Raw
  • K. R. Poeppelmeier
  • G. Trimarchi
  • H. Peng
  • J. Im
  • A. J. Freeman
  • N. H. Perry
  • T. O. Mason
  • A. Zakutayev
  • P. F. Ndione
  • D. S. Ginley
  • J. D. Perkins
چکیده

The structures of αand β-Ag3VO4 were studied via singlecrystal X-ray diffraction (XRD). The transition from α-phase to β-phase was found to occur at 110 °C. Single-crystal XRD revealed that the integrity of the single crystals was maintained as Ag3VO4 reversibly transitioned between α-Ag3VO4 and β-Ag3VO4. The optical and electrical properties of polycrystalline α-Ag3VO4 were studied by diffuse reflectance spectroscopy and impedance spectroscopy. In order to assess the optical and electrical properties of β-Ag3VO4, in situ measurements were performed above the phase-transition temperature. Thin films of α-Ag3VO4 were prepared by combinatorial sputtering and pulsed laser deposition (PLD). The crystallographic, optical, and electrical conductivity properties of the α-Ag3VO4 thin films were compared with the bulk properties.

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تاریخ انتشار 2012